Jun-Won Rhim

The anomalous Hall conductivity (AHC) in magnetic materials, resulting from inverted band topology, has emerged as a key adjustable function in spin‐torque devices and advanced magnetic sensors. Among systems with near‐half‐metallicity and broken time‐reversal symmetry, cobalt disulfide (CoS 2 ) has proven to be a material capable of significantly enhancing its AHC. In this study, the AHC of CoS 2 is empirically assessed by manipulating the chemical potential through Fe‐ (hole) and Ni‐ (electron) doping. The primary mechanism underlying the colossal AHC is identified through the application of density functional theory and tight‐binding analyses. The main source of this substantial AHC is traced to four spin‐polarized massive Dirac dispersions in the k z = 0 plane of the Brillouin zone, located slightly below the Fermi level. In Co 0.95 Fe 0.05 S 2 , the AHC, which is directly proportional to the momentum‐space integral of the Berry curvature (BC), reached a record‐breaking value of 2507 Ω −1 cm −1 . This is because the BCs of the four Dirac dispersions all exhibit the same sign, a consequence of the d ‐wave‐like spin‐orbit coupling among spin‐polarized e g orbitals.