Randall V. Martin

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Articles (11)

Year:

2023

Year:

2023

Year:

2023

Year:

2023

Year:

2023

Year:

2023

Year:

2023

Year:

2023

Year:

2022

A robust method to estimate mineral dust mass in ambient particulate matter (PM) is essential, as the dust fraction cannot be directly measured but is needed to understand dust impacts on the environment and human health. In this study, a global‐scale dust equation is developed that builds on the widely used Interagency Monitoring of Protected Visual Environments (IMPROVE) network's “soil” formula that is based on five measured elements (Al, Si, Ca, Fe, and Ti). We incorporate K, Mg, and Na into the equation using the mineral‐to‐aluminum (MAL) mass ratio of (K 2 O + MgO + Na 2 O)/Al 2 O 3 and apply a correction factor (CF) to account for other missing compounds. We obtain region‐specific MAL ratios and CFs by investigating the variation in dust composition across desert regions. To calculate reference dust mass for equation evaluation, we use total‐mineral‐mass (summing all oxides of crustal elements) and residual‐mass (subtracting non‐dust species from total PM) approaches. For desert dust in source regions, the normalized mean bias (NMB) of the global equation (within ±1%) is significantly smaller than the NMB of the IMPROVE equation (−6% to 10%). For PM 2.5 with high dust content measured by the IMPROVE network, the global equation estimates dust mass well (NMB within ±5%) at most sites. For desert dust transported to non‐source regions, the global equation still performs well (NMB within ±2%). The global equation can also represent paved road, unpaved road, and agricultural soil dust (NMB within ±5%). This global equation provides a promising approach for calculating dust mass based on elemental analysis of dust.

Year:

2022

Year:

2022

Collaborators (9)

Jeffrey R. Pierce

-

UNITED STATES
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Klaas Boersma

Associate Professor

Wageningen Universiteit

NETHERLANDS
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Daniel Bogale Odo

Australian National University

AUSTRALIA
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Ronald C. Cohen

University of California

UNITED STATES
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JUN MENG

Assistant Professor

Washington State University

UNITED STATES
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Jay Kaufman

Professor

McGill University

CANADA
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Rachel Ying-Wen Chang

Associate Professor

Dalhousie University

CANADA
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Jeffrey C Kwong

University of Toronto

CANADA
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Heresh Amini

Københavns Universitet

DENMARK
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